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ARM Expands Collection of Aerosol Mass Concentration Data Sets

Published: 17 November 2025

The title of the plot is BNF ToF-ACSM data corrected for CDCE. The y-axis represents mass loading (ug/m^3) from 0 to 14, while the x-axis represents June 1 through 15, 2025, showing how the mass loading changes over time with organics (green line), ammonium (gold line), sulfate (red line), and nitrate (blue line). Organics dominate the plot well above the other lines.
This sample plot from ARM’s Bankhead National Forest (BNF) atmospheric observatory shows a selection of aerosol mass concentrations corrected for composition-dependent collection efficiency. Plot was generated by Maxwell Levin, Pacific Northwest National Laboratory.

The Atmospheric Radiation Measurement (ARM) User Facility recently released new data from the Aerosol Chemical Speciation Monitor (ACSM) Composition-Dependent Collection Efficiency (CDCE) value-added product (ACSMCDCE VAP).

The ACSMCDCE VAP implements a procedure described by Middlebrook et al. (2012) to correct ACSM aerosol mass concentration data for CDCE, or non-unity detection of particle mass by the instrument. This improves the accuracy of the ACSM data and brings them into better agreement with other colocated aerosol measurements.

ARM produces ACSMCDCE for its quadrupole and time-of-flight (ToF) ACSMs, which use different mass spectrometers to separate ions by their mass-to-charge ratio. The ToF instrument is newer technology and has better (lower) detection limits than the quadrupole ACSM.

The ACSMCDCE VAP is now in production for three new ARM sites:

In addition, historical ACSMCDCE data are now available for:

The BNF main site and NSA E30 have ToF-ACSMs, so an ACSMTOFCDCE c1-level data product is available for those sites. Quadrupole ACSMCDCE c1-level VAP data are available for the other sites.

More information about the data, including the technical report, is available on the ACSMCDCE web page.

Scientists can access the new data now in the ARM Data Center. (To download the data, first create an ARM account.)

Please contact ARM translator John Shilling or VAP developer Maxwell Levin to ask questions, report data issues, or provide feedback to help improve these data.

Data can be referenced as doi:10.5439/1641833 for the quadrupole ACSMCDCE data and doi:10.5439/1878136 for ACSMTOFCDCE.

Reference: Middlebrook AM, R Bahreini, JL Jimenez, and MR Canagaratna. 2012. “Evaluation of Composition-Dependent Collection Efficiencies for the Aerodyne Aerosol Mass Spectrometer using Field Data.” Aerosol Science and Technology, 46(3):258-271, https://doi.org/10.1080/02786826.2011.620041

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ARM is a DOE Office of Science user facility operated by nine DOE national laboratories.

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Atmospheric Radiation Measurement (ARM) | Reviewed March 2025